Can I Use PS3 Controller on Xbox 360?
Nope, a PS3 controller won't work directly on an Xbox 360. They're like cats and dogs; they just don't get along natively.
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You'd need a special adapter to make a PS3 controller work on an Xbox 360. It's a bit of a hassle, but totally doable!
Short answer: No. Different systems, different controllers.
I've tried using a PS3 controller on my Xbox 360 before. You'll need a controller converter, like the CronusMAX or Titan One. Worked decently for me!
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