Can you leave the Brotherhood in Fallout 4?
Yeah, you can totally bail on the Brotherhood of Steel in Fallout 4. Just make a decision that goes against their ideals or get cozy with another faction that they don't like. For example, helping out the Railroad or the Institute is a surefire way to get on their bad side. Just be ready for a bit of hostility once you make your break!
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Short answer: Yes. Decisions matter in Fallout 4, and aligning with other factions can naturally lead you away from the Brotherhood.
Absolutely, I did it in my last playthrough. Just got involved with the Railroad and next thing I know, BoS wasn't too happy with me. It's all about the choices you make and who you decide to support.
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