How to Turn Off PS3 Controller on PC
Just hold the PS button for about 10 seconds, and it should turn off. Easy peasy!
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Unplugging the USB cable works like a charm for me!
Using Bluetooth? Head to the Bluetooth settings on your PC and hit 'disconnect' for the PS3 controller.
You can use a third-party tool like SCP Toolkit, which gives you an option to disconnect the controller via the software.
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