How to Use PS Vita as PS3 Controller
Easy peasy! On your PS Vita, go to the Remote Play app and link it with your PS3. Once linked, you can use the PS Vita as a controller.
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Honestly, the PS Vita isn't great as a PS3 controller. Just get a DualShock 3 for the best experience.
Just connect your PS Vita to the PS3 via the Remote Play feature. It's simple and works pretty well!
Go to the Remote Play settings on your PS3, then pair it with your PS Vita. Use the Remote Play app on the Vita, and voil脿, you're good to go!
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